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You are able to buy "Caillou - Season 1" on Apple TV as download.
There are no options to watch Caillou for free online today in Canada. You can select 'Free' and hit the notification bell to be notified when season is available to watch for free on streaming services and TV.
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From PBS KIDS - Meet Caillou, the lovable 4-year-old with a big imagination! Caillou experiences all the wonders of being a child that audiences around the world can relate to; first day of school, caring for a pet, learning a new sport, or spending time with family. Preschoolers feel right at home with trusted pal Caillou, his sister Rosie, and all their family and friends as they experience the everyday adventures of childhood.