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Currently you are able to watch "The Smurfs" streaming on Netflix. It is also possible to buy "The Smurfs" on Apple TV as download or rent it on Apple TV online.
When the evil wizard Gargamel chases the tiny blue Smurfs out of their village, they tumble from their magical world and into ours -- in fact, smack dab in the middle of Central Park. Just three apples high and stuck in the Big Apple, the Smurfs must find a way to get back to their village before Gargamel tracks them down.