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You are able to buy "Caillou - Season 1" on Apple TV as download.
Caillou is available to watch for free today. If you are in Australia, you can:
Growing up is the greatest adventure, especially when you are 4 years old. Each Caillou episode is about a simple everyday life situation that feels so BIG to a child. It's about discovery and imagination. Watching Caillou helps children feel empowered and inspired. What Caillou does in the episodes reflects what every child does in their day-to-day lives.